宁宁1,, 房文汇1,2,*, 郑浩财1,, 容广健1,, 张喜和1,, 胡婷婷1,
( 1、长春理工大学理学院,长春 130022; 2、吉林大学物理学院,长春 130022; )
摘要: 利用激光诱导击穿效应在二硫化碳中获得了硫二相(S-Ⅱ)的受激拉曼散射光谱(SRS)。当激光强度大于液体的击穿阈值时,将产生冲击波,同时伴随产生动高压和温度场。实验获得了S-Ⅱ相的289cm-1的E弯曲振动模式和490cm-1的A1对称伸缩振动模式。当强冲击波产生的压强和温度场处于S-Ⅱ相的稳态范围时,激光分解产生了S-Ⅱ相的结构。激光诱导击穿所引发的高动态压强和静电场使A1振动模式频移变大。
关键词: 光学;等离子体;受激拉曼散射
NING Ning1,, FANG Wenhui1,*, ZHENG Haocai2,, RONG Guangjian1,, ZHANG Xihe1,, HU Tingting1,
( 1、School of Science,Changchun University Of Science And Technology,Changchun 130022; 2、College of Physics,Jilin University,Changchun 130022; )
Abstract: The study of Stimulated Raman scattering (SRS) of sulfur-II (S-II) phase was investigated by laser decomposition of carbon disulfide.The carbon disulfide was existed as liquid. Above a threshold of the laser intensity, it is suggested. A strong shock wave is generated in the liquid carbon disulfide, which is decomposed owing to the induced high dynamic pressure and temperature. One bending mode E frequency at 289 cm?1 and one symmetric stretching mode A1 frequency at 490 cm?1 of S-II phase were observed. The SRS spectra indicated that S-II structure is formed by laser decomposition, because of the strong shock wave generates the stable pressure-temperature range of S-II phase. The dynamic highpressure and static-electric field generated by laser-induced breakdown results in the softening A1 mode becoming more hardened.
Keywords: optics; plasma; Stimulated Raman Scattering
作者简介: 宁宁(1990-),女,硕士研究生,激光与物质相互作用
通信联系人: 房文汇(1982-),女,长春理工大学理学院讲师、硕士研究生副导师,主要研究方向:分子光谱学、激光与物质相互作用。从事激光与物质相互作用,分子光谱学研究多年,完成并参与国家自然科学基金、吉林省科技厅青年基金、博士后科学基金、吉林省教育厅科研项目等多项科研课题,发表科研论文20余篇
中国科技论文在线:宁宁,房文汇,郑浩财等. 激光诱导二硫化碳分解及硫-Ⅱ相的受激拉曼散射研究[EB/OL].北京:中国科技论文在线 [2016-07-26].http://www.paper.edu.cn/releasepaper/content/201607-256.
发表期刊: http://www.lunwenbang.com/